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This clear and self-contained review of the last four decades of research highlights in the hot field of nonlinear optical (NLO) crystals, particularly of borate-based ultraviolet and deep-ultraviolet NLO crystals, covers three major subjects: the structure-property relationship in borate crystals, the structural and optical characteristics of various promising borate crystals, and their fruitful applications in a wide range of scientific and technological fields. Edited by the discoverers and users of these optical borate crystals, this is a readily accessible reading for semiconductor, a