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2Philogos
I started with Sapiens. I found Homo Deus reused a lot of material so, although it does go further, you end up seeing a lot of the same stuff from a different angle. There is new stuff, particularly towards the end and, as I said, the approach is a bit different so I'd say that reading both is actually worthwhile, especially if you enjoy his style.
3Tytania
21 LESSONS FOR THE 21ST CENTURY is his latest and was definitely worthwhile. I read SAPIENS first and it was one of the best books I ever read, thus hard to top. HOMO DEUS & 21 LESSONS kind of continue with the same themes, so it wasn't as life-disrupting to read them, but he's definitely become one of my favorite authors and thinkers.

